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Reaction-driven surface restructuring and selectivity control in allylic alcohol catalytic aerobic oxidation over Pd

Lee, Adam Fraser, Ellis, Christine Victoria, Naughton, James N., Newton, Mark A., Parlett, Christopher Michael A. and Wilson, Karen 2011. Reaction-driven surface restructuring and selectivity control in allylic alcohol catalytic aerobic oxidation over Pd. Journal of the American Chemical Society 133 (15) , pp. 5724-5727. 10.1021/ja200684f

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Abstract

Synchronous, time-resolved DRIFTS/MS/XAS cycling studies of the vapor phase selective aerobic oxidation of crotyl alcohol over nanoparticulate palladium reveal surface oxide as the desired catalytically active phase, with dynamic, reaction-induced palladium redox processes controlling selective versus combustion pathways.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Cardiff Catalysis Institute (CCI)
Chemistry
Subjects: Q Science > QD Chemistry
Publisher: American Chemical Society
ISSN: 0002-7863
Last Modified: 03 Apr 2018 20:34
URI: http://orca-mwe.cf.ac.uk/id/eprint/9644

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