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Base-free oxidation of glucose to gluconic acid using supported gold catalysts

Cao, Yeuling, Liu, Xi, Iqbal, Sarwat, Miedziak, Peter John, Edwards, Jennifer Kelly, Armstrong, Robert, Morgan, David John, Wang, Junwei and Hutchings, Graham John 2015. Base-free oxidation of glucose to gluconic acid using supported gold catalysts. Catalysis Science & Technology 6 , pp. 107-117. 10.1039/C5CY00732A

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Abstract

1%Au/TiO2 catalysts prepared by a range of preparation methods were studied for the base-free oxidation of glucose. The highest catalytic activity was observed with the catalyst prepared by the sol-immobilization method. Furthermore we have studied the effect of the post-synthesis treatments of treatment with water, or heating in air on the activity. The catalyst calcined at 250 °C showed optimal activity and selectivity. Additionally, we studied the effect of the amount of the stabilising ligand in the sol-immobilisation method and observed that this is a key parameter with respect to determining catalyst activity.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Cardiff Catalysis Institute (CCI)
Chemistry
Subjects: Q Science > QD Chemistry
Publisher: Royal Society of Chemistry
ISSN: 2044-4753
Funders: European Research Council
Date of First Compliant Deposit: 30 March 2016
Date of Acceptance: 22 August 2015
Last Modified: 20 May 2019 21:37
URI: http://orca-mwe.cf.ac.uk/id/eprint/76060

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