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In-situ x-ray studies of clean catalytic technologies

Lee, Adam Fraser, Ellis, Christine Victoria, Newton, Mark A., Parlett, Christopher Michael A. and Wilson, Karen 2011. In-situ x-ray studies of clean catalytic technologies. Presented at: Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies, San Francisco, CA, USA, 25 - 29 April 2011. Published in: Tao, F., Salmeron, M., Rodriguez, J. A. and Hu, J. eds. 2011 MRS Spring Meeting - Symposium FF – Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies. MRS Proceedings , vol. 1351. Cambridge: Cambridge University Press, 10.1557/opl.2011.1170

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Abstract

The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

Item Type: Conference or Workshop Item (Paper)
Date Type: Publication
Status: Published
Schools: Chemistry
Cardiff Catalysis Institute (CCI)
Subjects: Q Science > QD Chemistry
Uncontrolled Keywords: Pd; oxidation; extended x-ray absorption fine structure(EXAFS)
Publisher: Cambridge University Press
ISBN: 9781605113289
ISSN: 1946-4274
Last Modified: 05 Jan 2018 22:03
URI: http://orca-mwe.cf.ac.uk/id/eprint/17371

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